| Voice Actor | Charlie Adler (as Natural "Nat" Smurfling (1985–1989)), Jack Angel (as Enchanter Homnibus (1982–1988)), Michael Bell (as Grouchy Smurf, Handy Smurf, Lazy Smurf, Johan (1982–1988)/Additional Voices), Lucille Bliss (as Smurfette), Susan Blu (as Nanny Smurf (1988), Pansy), William Callaway (as Clumsy Smurf, Painter Smurf/Additional Voices), Joey Camen (as Natural Smurf (1983–1985)), Hamilton Camp (as Greedy Smurf, Harmony Smurf, Woody/Additional Voices), William Christopher (as Angel Smurf), Keene Curtis (as Lord Balthazar), Jennifer Darling (as Princess Sabina), Marshall Efron (as Sloppy Smurf), June Foray (as Jokey Smurf/Mother Nature/Gargamel's Mother/Additional Voices), Richard Gautier (as Wooly Smurf), Danny Goldman (as Brainy Smurf), Bob Holt (as The King (1982–1985)), Arte Johnson (as Devil Smurf), Don Messick (as Papa Smurf, Azrael, Dreamy Smurf, Sickly Smurf (1983), Sweepy Smurf/Additional Voices), Julie McWhirter (as Baby Smurf (1986–1989), Sassette Smurfling (1985–1989)), Kris Stevens (as The Narrator (1981–1985)), Paul Kirby (as The Narrator (1985-1989)), Frank Welker (as Hefty Smurf, Clockwork Smurf, Peewit (1982–1989), Poet Smurf, Puppy (1985–1988), Wild Smurf (1987–1989), Nemesis (1988), Darkness Monster, Sandman/Additional Voices), Paul Winchell (as Gargamel, Baby Smurf, Nosey Smurf), Jonathan Winters (as Grandpa Smurf (1986–1989)) |
